The antioxidant and chlorogenic acid profiles of whole coffee fruits are influenced by the extraction procedures

  • W. Mullen
  • , B. Nemzer
  • , B. Ou
  • , A. Stalmach
  • , J. Hunter
  • , M. N. Clifford
  • , E. Combet

Research output: Contribution to journalArticlepeer-review

98 Citations (Scopus)

Abstract

Commercial whole coffee fruit extracts and powder samples were analyzed for chlorogenic acids (CGA), caffeine and antioxidant activities. CGA and caffeine were characterized by LC-MSn and HPLC accordingly, and quantified by UV absorbance. ORAC, HORAC, NORAC, SORAC and SOAC (antioxidant capacities) were assessed. Three caffeoylquinic acids, three feruloylquinic acids, three dicaffeoylquinic acids, one p-coumaroylquinic acid, two caffeoylferuloylquinic acids and three putative chlorogenic lactones were quantified, along with a methyl ester of 5-caffeoylquinic acid (detected in one sample, the first such report in any coffee material). Multistep whole coffee fruit extracts displayed higher CGA content than single-step extracts, freeze-dried, or air-dried whole raw fruits. Caffeine in multistep extracts was lower than in the single-step extracts and powders. Antioxidant activity in whole coffee fruit extracts was up to 25-fold higher than in powders dependent upon the radical. Total antioxidant activity of samples displayed strong correlation to CGA content.

Original languageEnglish
Pages (from-to)3754-3762
Number of pages9
JournalJournal of Agricultural and Food Chemistry
Volume59
Issue number8
DOIs
Publication statusPublished - 27 Apr 2011

Keywords

  • antioxidant activity
  • caffeine
  • chlorogenic acid
  • coffee fruits
  • extract
  • green coffee

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